The 25-year-old wrote the music for new British film Submarine, out this Friday in the UK, and now wants to take on the job of doing the 007 theme tune.
Speaking at the London premiere of comedy Submarine, he told BBC 6 Music he is up for further film work - but only selected projects.
He said: 'I don't think I'd be very good at doing the soundtrack for Transformers or anything like that.'
But when asked if he'd do a James Bond theme, the rocker said: 'Well, that's a different story. I'd love to do a tune for Bond. Definitely.'